Abstract
Correlations in systems with spin degree of freedom are at the heart of fundamental phenomena, ranging from magnetism to superconductivity. The effects of correlations depend strongly on dimensionality, a striking example being one-dimensional (1D) electronic systems, extensively studied theoretically over the past fifty years1,2,3,4,5,6,7. However, the experimental investigation of the role of spin multiplicity in 1D fermions—and especially for more than two spin components—is still lacking. Here we report on the realization of 1D, strongly correlated liquids of ultracold fermions interacting repulsively within SU(N) symmetry, with a tunable number N of spin components. We observe that static and dynamic properties of the system deviate from those of ideal fermions and, for N > 2, from those of a spin-1/2 Luttinger liquid. In the large-N limit, the system exhibits properties of a bosonic spinless liquid. Our results provide a testing ground for many-body theories and may lead to the observation of fundamental 1D effects8.
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One-dimensional quantum systems show specific, sometimes counterintuitive behaviours that are absent in the 3D world. These behaviours, predicted by many-body models of interacting bosons9 and fermions2,3,4, include the ‘fermionization’ of bosons10 and the separation of spin and density (most commonly referred to as ‘charge’) branches in the excitation spectrum of interacting fermions. The last phenomenon is predicted within the celebrated Luttinger liquid model5, which describes the low-energy excitations of interacting spin-1/2 fermions. Although the Luttinger approach describes qualitatively the physics of a number of 1D systems11,12, the problem of how to extend it to a more detailed description of real systems has puzzled physicists over the years7. In this exploration the physics of spin has played a key role.
Ultracold atoms have proved to be a precious resource to study 1D physics, as they afford exceptional control over experimental parameters. Most of the experiments so far have been performed with spinless bosons, which for instance led to the realization of a Tonks–Girardeau gas13,14. On the other hand, 1D ultracold fermions are a promising system to observe a number of elusive phenomena, such as Stoner’s itinerant ferromagnetism15 and the physics of spin-incoherent Luttinger liquids6. However, only a few pioneering works, dealing with spin-1/2 particles16,17,18, have been reported so far.
In parallel, ultracold two-electron atoms have been recently proposed for the realization of large-spin systems with SU(N) interaction symmetry19,20, and the first experimental investigations have been reported21. This novel platform enables the simulation of 1D systems with a high degree of complexity, including spin–orbit-coupled materials22 or SU(N) Heisenberg and Hubbard chains23,24. Moreover, the investigation of these multi-component fermions is relevant for the simulation of field theories with extended SU(N) symmetries25.
In this Letter we report on the realization of 1D quantum wires of repulsive fermions with a tunable number of spin components, which are created by tightly trapping ultracold 173Yb atoms in a 2D optical lattice (Fig. 1a). The purely nuclear spin I = 5/2 of 173Yb results both in the independence of the interaction strength from the nuclear spin state and in the absence of spin-changing collisions. The latter feature is particularly important for our experiments, as it implies the stability of any spin mixture. The atoms experience an axial harmonic confinement with (angular) frequency ωx ≈ 2π × 80 Hz and a strong radial confinement with ω⊥ = 2π × 25 kHz, resulting in the occupation of the radial ground state. We use optical spin manipulation and detection techniques (see Supplementary Information) to prepare the system in an arbitrary number N ≤ 2I + 1 = 6 of spin components (Fig. 1b), thus realizing different SU(N) symmetries. We directly compare systems with different N, keeping the atom number per spin component Nat ≃ 6,000 (≈20 atoms per spin component in the central wire) and all the other parameters constant. This approach enables us to examine how the physics of a strongly-interacting 1D fermionic system changes as a function of N.
Momentum distribution
We investigate the correlations in the 1D wires by observing the momentum distribution n(k) (k is the momentum divided by the reduced Planck’s constant ħ). We measure this quantity by extinguishing the trapping light and imaging the atomic cloud after a ballistic expansion, as done in previous works to measure n(k) of a Tonks–Girardeu gas13. A typical image is reported in Fig. 2c, where denotes the wire axis. Integration over results in the n(k) curves plotted in Fig. 2a for different N (the curves are normalized to have the same unit area). In the non-interacting case N = 1 the data (solid blue) are very well accounted for by the theory of a trapped ideal Fermi gas (dashed blue, see Supplementary Information). Increasing N, we observe a clear monotonic broadening of n(k), with a reduction of the weight at low k and a slower decay of the large-k tails.
The observed n(k) broadening arises from a pure effect of correlations that goes beyond standard mean-field physics. To give a qualitative understanding of this phenomenon, we consider spin-1/2 fermions with infinite repulsion. In this limit, the density–density correlation function (where and are the density operators for the two spin components) falls to zero for d → 0 as G↑ ↑(d) does in the case of a spin-polarized gas, thus mimicking the effects of Pauli repulsion between distinguishable particles. This ‘fermionization’, restricting the effective space which is available to the particles, causes them to populate states with larger momentum26,27. We note that an opposite behaviour would be predicted by a mean-field treatment of interactions neglecting correlations between trapped fermions: the effectively weaker confinement along induced by the atom-atom repulsion would lead to more extended single-particle wavefunctions, hence to a decreased width of n(k) (Fig. 2b). For N = 2 the interaction regime of our 1D samples is described by the parameters γ ≃ 4.8 and K ≃ 0.73 (see Supplementary Information), lying in the strongly-correlated regime between the ideal Fermi gas (γ = 0, K = 1) and a fully fermionized gas (γ = ∞, K = 0.5).
The details of n(k) depend nontrivially on the temperature, owing to the thermal population of spin excitations. The temperature regime for our experiments, T ≃ 0.3 TF (where TF is the Fermi temperature), is slightly below the predicted temperature scaleTS ≃ 0.4 TF for spin excitations (see Supplementary Information), in the crossover between the spin-ordered regime for T ≪ TS and that of a spin-incoherent Luttinger liquid for T ≫ TS (ref. 6). Fig. 2b shows the theoretical n(k) for N = 2 and infinite repulsion in the limiting regimes T = 0 and T ≫ TS (light and dark solid curves, derived from refs 26 and 27, respectively). Although both curves show an evident n(k) broadening, in accordance with our observations, their shape is different and can be explained in terms of a modified effective Fermi momentum28. Exact calculations for finite interactions and finite temperatures are challenging, thus making our system a profitable quantum simulation resource for the fundamental problem of 1D interacting fermions.
Probing excitations
A distinctive feature of 1D fermions is the existence of a well-resolved excitation spectrum at small momenta ħ q ≪ ħ kF (where kF is the Fermi wave vector). Number-conserving excitations in the ideal 1D Fermi gas correspond to particle–hole pairs with energy ħ ω = vFħ q, where vF = ħ kF/m is the Fermi velocity (Fig. 3a, inset). This physical picture changes in the case of an interacting spin mixture, as excitations acquire a purely collective nature. According to the Luttinger theory, the spectrum of phononic excitations is still described by a linear dispersion ω = c q, where c = vF/K is a renormalized sound velocity1. In a two-component Luttinger liquid with contact repulsion one has 0.5 < K < 1. This yields a sound velocity that is larger than vF (Fig. 3b, inset), corresponding to an increased stiffness of the many-body state.
We have characterized the excitations of the fermionic wires by performing Bragg spectroscopy. This technique, relying on inelastic light scattering, allows the selective excitation of density waves with energy ħ ω and momentum ħ q (see Supplementary Information). Fig. 3a shows the measured spectrum for N = 1 at low momentum transfer ħ q ≃ 0.2 ħ kF0 (with kF0 being the peak Fermi wave vector in the central wire). A clear resonance is observed, in excellent agreement with the calculated response for ideal fermions (solid line, with no free parameters). For N = 2 the resonance is clearly shifted towards higher frequencies (Fig. 3b), as expected from the Luttinger theory. The measured shift (+15 ± 4)% agrees with the expected (+10 ± 2)% shift in the sound velocity predicted on the basis of the Luttinger theory for a trapped system (see Supplementary Information). For N = 6 the spectrum shows a much larger shift (+33 ± 4)% (Fig. 3c), which disagrees with the predictions for N = 2, signalling an increased effect of interactions, in qualitative accordance with the n(k) change of Fig. 2. We also plot the calculated spectra for trapped fermions with infinite interactions (Fig. 3b,c, dotted lines), which shows how the measured spectra lie between the response of the ideal Fermi gas and that of a fermionized system.
Collective mode frequencies
More insight into the physics of multicomponent 1D fermions can be gained by studying low-energy breathing oscillations in which the cloud radius oscillates in time. We measure the frequency of this collective mode by suddenly changing the trap frequency and measuring the time evolution of the radius. In Fig. 4a we plot the measured squared ratio β = (ωB/ωx)2 of the breathing frequency ωB to the trap frequency ωx as a function of N (squares). For N = 1 the measured value is in good agreement with the expected value β = 4 for ideal fermions (upper horizontal line). With increasing N our data clearly show a monotonic decrease of β, induced by the repulsive interactions in the spin mixture.
The dependence of β on the interaction strength is remarkably nontrivial, already for N = 2, as first predicted in ref. 29. Indeed, β = 4 in both the limiting cases of an ideal gas (γ = 0) and a fermionized (γ = ∞) system, whereas for finite repulsion it is expected to exhibit a nonmonotonic behaviour, with a minimum at finite interaction strength. The theoretical curves in Fig. 4b show the expected dependence of β on the interaction parameter η = Nat1(a1D/ax)2 (where Nat1 is the number of atoms per wire, a1D is the 1D scattering length and ax is the trap oscillator length). We have derived these results by combining a Bethe Ansatz approach with the exact solution of the hydrodynamic equations describing a 1D fermionic liquid with N components (see Supplementary Information). As N is increased, the curves exhibit an increasingly larger redshift of β, and for N →∞ they asymptotically approach the curve for 1D spinless bosons. The circles indicate the theoretical values for the average η = 0.44 in our experiment. The agreement between experiment and theory is excellent, as shown in Fig. 4a (we note that for N = 2 both theory and experiment agree with the results of ref. 29).
The experimental data, accompanied by our theoretical curves, clearly show that changing N causes markedly different effects from those induced by simply changing the interaction strength in an N = 2 mixture. In fact, by increasing N, the constraints of the Pauli principle become less stringent and the number of binary-collisional partners increases, causing the system to acquire a more ‘bosonic’ behaviour. Our experimental value at N = 6 clearly falls out of the range of β expected for an N = 2 liquid (Fig. 4, grey regions), and already approaches the value expected for 1D spinless bosons. This bosonic limit for N →∞ is a remarkable property of multi-component 1D fermions that has been pointed out theoretically only very recently30 and that our experimental system is capable to clearly evidence.
Concluding remarks
The possibility of tuning the number of spin components allows us to study different regimes of interplay between Fermi statistics and the degree of distinguishability in this novel 1D system. From a quantum simulation perspective, this realization provides a powerful test bench for large-spin models and opens a route towards the investigation of fundamental effects ranging from spin dynamics to novel magnetic phases.
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Acknowledgements
We would like to thank all the members of the Ultracold Quantum Gases group in Florence for fruitful discussions. We are indebted to P. Calabrese for enlightening discussions on the physics of 1D quantum systems, and to P. Cancio, G. Giusfredi and P. De Natale for early valuable contributions to the experimental set-up. We also thank M. Dalmonte A. Recati and M. Polini for valuable discussions. This work has been financially supported by IIT Seed Project ENCORE, ERC Advanced Grant DISQUA, EU FP7 Integrated Projects AQUTE and SIQS, MIUR Project PRIN2009, ARC Discovery Projects (Grants No. DP0984522 and No. DP0984637) and NFRP-China (Grant No. 2011CB921502).
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All authors contributed to the writing of the manuscript. G.P., M.M., G.C., P.L., F.S., J.C., C.S., M.I. and L.F. built the experimental set-up, performed the measurements and analysed the data. H.H. and X-J.L. carried out the theoretical derivation of the breathing frequencies.
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Pagano, G., Mancini, M., Cappellini, G. et al. A one-dimensional liquid of fermions with tunable spin. Nature Phys 10, 198–201 (2014). https://doi.org/10.1038/nphys2878
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DOI: https://doi.org/10.1038/nphys2878
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